The title track from "Ride the Lightning". I used to love to listen to this track and album while snowboarding.
http://www.youtube.com/watch?v=uebInqG1pJI
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Nothing Else Matters.

By far the greatest song from them. Always brings back memories from easier times ;)
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I used to be a Metallica freak! There are many tracks I love, but "Unforgiven" was my favorite of all time because it seemed to speak to me personally. Anyone remember when that album came out back in the early 1990's? My husband and I had a disagreement. He said "Enter Sandman" was originally the most popular track from that album, but I disagree. "Unforgiven" was the song I remember the radio stations started playing immediately and "Enter Sandman" was added to the playlists later on.

Now, however, I have lost respect for Metallica due to their voicing such opposition about downloading their music online. I think they should just be psyched that so many people love their music. I mean, seriously, they already make millions each year. They have to be one of the highest paid groups ever and they are griping? So, I haven't bought a Metallica album in almost ten years now.
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I have never been a fan of "Hard" or "Metal" rock, but "Enter Sandman" was a song that I caught myself hooked on. So I would have to say, Enter Sandman.
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Enter Sandman

http://www.bing.com/videos/search?q=enter+sandman&qpvt=enter+sandman&FORM=Z7FD1

http://en.wikipedia.org/wiki/Enter_Sandman
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Fade to Black, from the Ride the Lightning record.
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I like "no leaf clover" from the S&M album
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