I think the best video screen capture software for the Mac is Screenflow from Telestream, Inc. They have a trial so you can see what you get before you buy, and an iPhone app as well. I used the software a while back, but remember I was impressed with the features. I will put a link in the resources below.

On the PC, I've used Camtasia for years, and I like that a lot. They make it very easy to use as well. Camtasia announced that they will have a version for the Mac out in mid 2009. Again, I've included some links to that info in the resources area of this post.
Source(s):
Screenflow by Telestream
http://www.telestream.net/screen-flow/overview.htm

Camtasia (soon) for the Mac
http://www.techsmith.com/macdevelopment.asp and
http://visuallounge.techsmith.com/2009/01/camtasia_for_the_mac_update.html

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